Nonlinear Sensing with Whispering-Gallery Mode Microcavities: From Label-Free Detection to Spectral Fingerprinting
Author(s): Liu, WJ (Liu, Wenjing); Chen, YL (Chen, You-Ling); Tang, SJ (Tang, Shui-Jing); Vollmer, F (Vollmer, Frank); Xiao, YF (Xiao, Yun-Feng)
Source: NANO LETTERS Volume: 21 Issue: 4 Pages: 1566-1575 DOI: 10.1021/acs.nanolett.0c04090 Published: FEB 24 2021
Abstract: Optical microresonators have attracted intense interests in highly sensitive molecular detection and optical precision measurement in the past decades. In particular, the combination of a high quality factor with a small mode volume significantly enhances the nonlinear light-matter interaction in whispering-gallery mode (WGM) microresonators, which greatly boost nonlinear optical sensing applications. Nonlinear WGM microsensors not only allow for label-free detection of molecules with an ultrahigh sensitivity but also support new functionalities in sensing such as the specific spectral fingerprinting of molecules with frequency conversion involved. Here, we review the mechanisms, sensing modalities, and recent progresses of nonlinear optical sensors along with a brief outlook on the possible future research directions of this rapidly advancing field.
Accession Number: WOS:000624334100002
PubMed ID: 33356315
Author Identifiers:
Author Web of Science ResearcherID ORCID Number
Liu, Wenjing B-3816-2019 0000-0002-9441-8859
ISSN: 1530-6984
eISSN: 1530-6992
Full Text: https://pubs.acs.org/doi/10.1021/acs.nanolett.0c04090